The musician, from Kingston, Jamaica, was a founding member of The Wailers alongside his childhood friend, Bob Marley.
Together, they achieved international fame with reggae classics like Simmer Down and Stir It Up, before Wailer left to go solo in 1974.
He went on to win three Grammys and was given Jamaica's Order Of Merit in 2017.
His death was confirmed by manager Maxine Stowe, and Jamaica's Culture Minister, Olivia Grange.
The cause of death is unknown, but he had been in hospital since having a stroke in July 2020.
